Templated synthesis, postsynthetic metal exchange, and properties of a porphyrin-encapsulating metal-organic material

by Z. Zhang, L. Zhang, L. Wojtas, P. Nugent, M. Eddaoudi, M.J. Zaworotko
Year: 2012 DOI: 10.1021/ja209643b

Extra Information

J. Am. Chem. Soc., 134 (2), pp. 924-927, (2012)

Abstract

Reaction of biphenyl-3,4′,5-tricarboxylate (H 3BPT) and CdCl 2 in the presence of meso-tetra(N-methyl-4-pyridyl)porphine tetratosylate (TMPyP) afforded porph@MOM-10, a microporous metal-organic material containing CdTMPyP cations encapsulated in an anionic Cd(II) carboxylate framework, [Cd 6(BPT) 4Cl 4(H 2O) 4]. Porph@MOM-10 is a versatile platform that undergoes exchange to serve as the parent of a series of porph@MOMs that exhibit permanent porosity and heterogeneous catalytic activity.
 

Keywords

Metal exchange Metal-organic Microporous Porphine Templated synthesis Cadmium chloride Cadmium compounds Carboxylation Catalyst activity Porphyrins Synthesis (chemical) Cadmium Biphenyl 3 4' 5 tricarboxylate Carboxylic acid derivative Cation